Date of Award

Spring 1995

Document Type

Thesis - Restricted

Degree Name

Master of Science (MS)

Department

Mechanical Engineering

First Advisor

Brower, W. E.

Second Advisor

Fournelle, R. A.

Third Advisor

Blumenthal R. N.

Abstract

The rapid quenching of the Bi-Sr-Ca-cu-0 (2223) oxide was studied as a route to continuous production of the 2223 high Tc superconductors by forming in the glassy state. Rapid solidification of the as received BSCCO samples using the shock tube method resulted in the formation of partially glassy preforms in the region of the nominal 2223, the average composition of the flakes being Bi1.4Sr2 . 6Ca2Cu2.650y. The splat flakes were studied using different analytical methods, such as DSC, TMA, SEM with EDX, XRD, and Debye Scherrer powder diffraction technique. The flakes showed continuous flow in TMA (%penetration = 43-93%) and no melting endotherms or crystallization exotherms in DSC. Aggregates of flakes were partially glassy with additional precipitates of Cu, Cu20, and Cao. Results obtained by different analytical techniques were consistent and demonstrated that formable glass with the nominal 2223 composition could be prepared by the rapid solidification method.

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